ALD growth of MoS2 nanosheets on TiO2 nanotube supports

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dc.contributor.author Sopha, Hanna
dc.contributor.author Tesfaye, Alexander T.
dc.contributor.author Zazpe, Raul
dc.contributor.author Michalička, Jan
dc.contributor.author Dvořák, Filip
dc.contributor.author Hromádko, Luděk
dc.contributor.author Krbal, Miloš
dc.contributor.author Přikryl, Jan
dc.contributor.author Djenizian, Thierry
dc.contributor.author Macák, Jan
dc.date.accessioned 2019-08-08T10:07:21Z
dc.date.available 2019-08-08T10:07:21Z
dc.date.issued 2019-08-02
dc.identifier.issn 2452-2627
dc.identifier.uri https://hdl.handle.net/10195/73808
dc.description.abstract Two-dimensional MoS2 nanostructures are highly interesting and effective in a number of energy-related applications. In this work, the synthesis of ultra-thin MoS2 nanosheets produced by the thermal Atomic Layer Deposition (ALD) process is reported for the first time using a previously unpublished set of precursors. These nanosheets are homogenously deposited within one-dimensional anodic TiO2 nanotube layers that act as a high surface area conductive support for the MoS2 nanosheets. The decoration of high aspect ratio TiO2 nanotube layers with MoS2 nanosheets over the entire nanotube layer thickness is shown for the first time. The homogeneous distribution of the MoS2 nanosheets is proved by STEM/EDX. This resulting new composite is employed as anode for Li-ion microbatteries. The MoS2-decorated TiO2 nanotube layers show a superior performance compared to their counterparts without MoS2. A more than 50 % higher areal capacity and a coulombic efficiency of 98% are obtained on the MoS2 decorated TiO2 nanotube layers, demonstrating clear synergic benefits of the new composite structure. cze
dc.format p. eng
dc.language.iso en cze
dc.publisher Elsevier cze
dc.relation.ispartof FlatChem. August 2019
dc.rights Attribution-NonCommercial-NoDerivs 3.0 Czech Republic *
dc.rights.uri http://creativecommons.org/licenses/by-nc-nd/3.0/cz/ *
dc.subject TiO2 nanotube layers cze
dc.subject MoS2 cze
dc.subject nanosheets cze
dc.subject Atomic layer deposition cze
dc.subject Li-ion microbatteries cze
dc.title ALD growth of MoS2 nanosheets on TiO2 nanotube supports cze
dc.type Article cze
dc.event
dc.peerreviewed yes eng
dc.publicationstatus postprint eng
dc.identifier.doi 10.1016/j.flatc.2019.100130
dc.relation.publisherversion https://www.sciencedirect.com/science/article/pii/S2452262719300777?via%3Dihub
dc.project.ID EC/H2020/638857/EU/Towards New Generation of Solid-State Photovoltaic Cell: Harvesting Nanotubular Titania and Hybrid Chromophores/CHROMTISOL
dc.identifier.scopus 2-s2.0-85070354953


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Attribution-NonCommercial-NoDerivs 3.0 Czech Republic Except where otherwise noted, this item's license is described as Attribution-NonCommercial-NoDerivs 3.0 Czech Republic

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